In the search for unconventional magnetism, exotic quantum states are characterized by a lack of order and a broad spin excitation continuum approaching zero temperature. We study the two-dimensional triangular-lattice effective spin-Formula: see text system CeMgAl11O19, which shows slight disorder but no magnetic ordering down to 100 millikelvin. Spin-wave analysis in the magnetic-field-polarized state determines the spin Hamiltonian featuring a mixed ferromagnetic-antiferromagnetic nearest-neighbor exchange interaction [Formula: see text = -0.024(5) milli-electron volts, Formula: see text = 0.056(3) milli-electron volts]. This places the system near an exactly solvable point of the spin-Formula: see text triangular-lattice XXZ model (Formula: see text) with extensive ground-state degeneracy. In zero field, neutron spectroscopy reveals a prominent continuum; we show that this arises from an ensemble average of spin-wave spectra across the degenerate ground-state manifold. This demonstrates that the role of weak quenched disorder can be quantitatively constrained: It inhibits unique ground-state selection and stabilizes a local distribution within the degenerate manifold, yielding continuum-like spectra that necessitate a critical reevaluation of the experimental signatures of exotic quantum states.
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Bin Gao
T. Chen
Chunxiao Liu
Science Advances
University of California, Berkeley
Johns Hopkins University
Princeton University
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Gao et al. (Fri,) studied this question.
www.synapsesocial.com/papers/69ada892bc08abd80d5bbb3d — DOI: https://doi.org/10.1126/sciadv.aed7778