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October 2, 2025Journal of the American Chemical Society

Direct Deaminative Halogenation at Hindered Tertiary Centers

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Authors

ZCZhangkai CuiPMPanpan MaQSQi Sun

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Overview

This research demonstrates a novel approach to halogenation of α-tertiary amines, highlighting deaminative halogenation and functional group compatibility.

Key Points

  • The study showcases a radical-mediated approach for halogenation, simplifying reactions at crowded tertiary centers.
  • Efficient halogenation, including chlorination, bromination, and iodination, is achieved with diverse amine substrates.
  • The methodology opens pathways for late-stage molecular diversification with excellent functional group compatibility.
  • A broad substrate scope is combined with operational simplicity, potentially aiding drug candidate development.

Cite This Study

Cui et al. (2025) studied this question.

synapsesocial.com/papers/68de8eaeaa6cec72c69ea843https://doi.org/10.1021/jacs.5c13592
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