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February 2, 2026Crystals0 citationsOpen Access

To Study the Impact of Ultrasound-Assisted Antisolvent Crystallization on Aprepitant Crystal Habits

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APAditya PandhareLBLondhe Sachin BhimraoAAAtul Agrawal

Key Points

  • The aim is to evaluate how ultrasound-assisted antisolvent crystallization impacts the crystal habit of aprepitant.
  • Utilized solvent evaporation, conventional antisolvent crystallization, cooling crystallization, and sonocrystallization techniques.
  • Conducted morphological analysis and solid-state characterization including DSC, PXRD, and TGA.
  • Assessed wettability through contact angle measurements and intrinsic dissolution profiles.
  • Ultrasound-assisted crystallization produced smaller, platy crystals with improved micromeritics.
  • The APT_SN showed the highest tensile strength at 20 kg/cm2 among all crystal forms studied.
  • Modified crystals displayed improved powder properties and reduced intrinsic dissolution rates.

Abstract

Aprepitant (APT), an antiemetic drug used for chemotherapy-induced nausea and vomiting (CINV), exhibits poor compressibility, solubility, and micromeritic properties. Crystal habit modification was studied using solvent evaporation, conventional antisolvent crystallization (APTAS), cooling crystallization (APTCC), and the advanced sonocrystallization technique (APTSN). Morphological analysis of the sonocrystallized crystals revealed small, platy crystals exhibiting an aspect ratio of 1. 35 ± 0. 04 and a span value of 1. 06. The APTSN showed improved micromeritics as compared to APTAS (1. 59 ± 0. 03) and APTCC (1. 48 ± 0. 04) (antisolvent-crystallized APT and cooling crystallized APT, respectively). All modified crystals exhibited a plate-shaped crystal habit with no agglomeration. The angle of repose, Carr’s index, and Hausner’s ratio exhibit that the APTSN showed improvement in powder properties. Solid-state characterization using differential scanning calorimetry (DSC), Powder X-ray Diffraction Spectroscopy (PXRD), and Thermogravimetric Analysis (TGA) proved no change in polymorph. Contact angle-driven wettability was as follows: APT > APTAS > APTSN > APTCC, and the results were corroborated by X-ray photon spectroscopy (XPS) and intrinsic dissolution profiles. The XPS studies revealed a decrease in the surface polar component of APTSN, resulting in reduced wettability. APTSN showed the highest tensile strength at 20 kg/cm2 among all other crystals. All the modified crystals exhibited a reduced IDR profile, resulting from a reduction in the polar component at the surface.

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Cite This Study

Pandhare et al. (2026) studied this question.

synapsesocial.com/papers/6980fd81c1c9540dea80f3cbhttps://doi.org/10.3390/cryst16020096
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