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February 16, 2026Journal of Mass Spectrometry0 citationsOpen Access

HPLC‐MS/MS Method for Monitoring of L‐Asparaginase Activity by Using Asparagine and Aspartic Acid Plasma Levels

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CKCem KaplanİDİbrahim DANİŞDÜDurişehvar Özer Ünal

Key Points

  • To develop a method for monitoring L-asparaginase activity by analyzing plasma levels of asparagine, aspartic acid, and other related substrates.
  • Developed a high-performance liquid chromatography-tandem mass spectrometry method.
  • Analyzed plasma samples for asparagine, aspartic acid, glutamic acid, and L-glutamine.
  • Used acetonitrile and ammonium acetate in a gradient mobile phase flow at 0.4 mL/min.
  • Demonstrated linear amino acid detection range of 500-5000 ng/mL for asparagine and aspartic acid.
  • Achieved detection limits of 100-500 ng/mL for key amino acids in plasma samples.
  • Validated method proved to be selective and reproducible.

Abstract

ABSTRACT The effectiveness of L‐asparaginase and therefore the effectiveness of acute lymphoblastic leukemia treatment will be understood by determining the substrates of the enzyme, L‐asparagine and L‐glutamine. For this purpose, the high‐performance liquid chromatography–tandem mass spectrometry method was developed and validated by analyzing the L‐asparaginase substrates asparagine and glutamine and its products aspartic acid and glutamic acid from plasma. Acetonitrile and ammonium acetate were used at 0.4 mL/min in gradient mobile phase flow using a HILIC column for chromatographic separations. The linear amino acid range was found to be 500–5000 ng/mL for asparagine, aspartic acid, and glutamic acid, and 5–50 μg/mL for glutamine, respectively. Detection limit and quantitation limit were found to be 100–500 ng/mL for asparagine, aspartic acid, and glutamic acid, and 1–5 μg/mL for glutamine, respectively. The validated method has been successfully applied to plasma samples. The method was found to be selective and reproducible.

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Cite This Study

Kaplan et al. (2026) studied this question.

synapsesocial.com/papers/69926503eb1f82dc367a0e7fhttps://doi.org/10.1002/jms.70036
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