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February 22, 2026Advanced Materials0 citations

DNA Supramolecular Hydrogel Alters Exosomal microRNA Atlas and Paracrine Secretory Profile of MSCs to Promote Bone Remodeling and Ameliorate Osteoradionecrosis of the Jaw

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YLYanfang LiXLXue LiMQMiaomiao Qiu

Key Points

  • The aim is to enhance mesenchymal stem cell therapy for osteoradionecrosis by using a DNA supramolecular hydrogel.
  • Developed an injectable DNA supramolecular hydrogel as a 3D scaffold.
  • Assessed the retention of MSCs and their exosomes using the hydrogel over three weeks.
  • Evaluated the effects on the MSC secretome and microRNA profile through mechanotransduction pathways.
  • Prolonged local retention of MSCs and exosomes was confirmed for over three weeks.
  • The hydrogel modified the MSC secretome, shifting to a pro-regenerative exosomal miRNA profile.
  • In a murine model, it facilitated bone remodeling and improved tissue structure and inflammation.

Abstract

ABSTRACT Osteoradionecrosis of the jaw (ORNJ) is a severe complication of head and neck radiotherapy, characterized by a hostile tissue microenvironment that hinders healing. To address the limitations of mesenchymal stem cell (MSC) therapy, such as rapid dispersion and clearance, we developed an injectable, shear‐thinning DNA supramolecular hydrogel (DNASH) as a 3D scaffold. The DNASH matrix significantly prolonged the local retention of MSCs and their exosomes for over 3 weeks. Crucially, the scaffold actively reprogrammed the MSC secretome by modulating the FAK‑Integrin and Hippo‑YAP mechanotransduction pathways. This directed a shift toward a pro‐regenerative exosomal miRNA profile, notably enriching miR‑146a‑5p and reducing miR‑125b‑5p. In a murine ORNJ model, this MSC‐laden hydrogel orchestrated a coupled bone‐remodeling process, effectively clearing necrotic bone while stimulating robust osteogenesis. The treatment restored mandibular architecture, reduced systemic inflammation, and improved tissue homeostasis, presenting a clinically promising strategy for ORNJ repair.

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Cite This Study

Li et al. (2026) studied this question.

synapsesocial.com/papers/699a9d8e482488d673cd37f6https://doi.org/10.1002/adma.202523658
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