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February 25, 2026The Journal of Organic Chemistry0 citations

Regioselective Synthesis of 4,4′-Bipyrazoles via Palladium-Catalyzed Cyclizative Dimerization of Alkynic Hydrazones

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TKTaichi KusakabeHWHandong WangCTChizuru Torii

Key Points

  • The aim is to achieve regioselective synthesis of 4,4'-bipyrazoles through a palladium-catalyzed reaction.
  • Utilized palladium (Pd(tfa)<sub>2</sub>/DPPF) as a catalyst
  • Conducted dimerization of alkynic hydrazones
  • Tested various functional groups under reaction conditions
  • Successfully synthesized 4,4'-bipyrazoles with various substitutions
  • Demonstrated efficiency and tolerance for several functional groups

Abstract

Palladium-catalyzed cyclizative dimerization of alkynic hydrazones afforded 4,4'-bipyrazoles. The desired dimerization reaction proceeded efficiently by using the Pd(tfa)2/DPPF catalyst. Several functional groups were tolerated under the reaction conditions, and various bipyrazoles, including fully substituted bipyrazoles, were successfully synthesized.

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Cite This Study

Kusakabe et al. (2026) studied this question.

synapsesocial.com/papers/699e918df5123be5ed04f16ehttps://doi.org/10.1021/acs.joc.6c00022
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