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March 6, 20260 citationsOpen Access

Chirality Switching in 1T-TaS₂ by Highly Charged Ion Irradiation

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ANA. NiggasJBJens BuckDTD. Thima

Key Points

  • The aim is to explore chirality switching of charge density waves in 1T-TaS2 using high-energy accelerated ions.
  • Used Xe$^{8+}$ ions at 22.5 keV to irradiate 1T-TaS2
  • Conducted angle-resolved photoemission spectroscopy to monitor electronic properties
  • Performed experiments at a temperature of 50 K
  • Chirality switches gradually with ion fluence, reaching near-full reversal at ≳4000 ions/μm²
  • Changes in the band structure are most significant at charge density wave gaps
  • Ion-induced excitations are proposed to induce a phase transition leading to chiral switching.

Abstract

In layered materials, charge density waves can occur in distinct chiral phases, which can be switched. We use Xe^8+ ions at a kinetic energy of 22. 5 keV to switch the commensurate charge density wave chirality on the nanoscale in 1T-TaS₂ at 50 K. Changes in spectral weight, density of states, and band structure are monitored insitu by angle-resolved photoemission spectroscopy. We find that changes in the band structure are most pronounced at the charge density wave gaps and that chirality switches gradually with ion fluence, saturating to near-full handedness reversal at ≳4000 ions/μm². We discuss a scenario for ion-induced chiral switching within the framework of intense, spatially confined electronic excitations, which induce a phase transition and defect-stabilized grain boundaries.

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Cite This Study

Niggas et al. (2026) studied this question.

synapsesocial.com/papers/69aa7096531e4c4a9ff5a875https://doi.org/10.3204/pubdb-2026-00866
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