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March 10, 2026Chemical Engineering & Technology0 citations

Swelling Kinetics and Saponification‐Assisted Synthesis of Chitosan‐g‐PAA Superabsorbent Hydrogels

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JJayanudinRRahmayettyYMYenny Meliana

Key Points

  • The aim is to assess how alkali-assisted hydrolysis and crosslinking affect the swelling properties of chitosan-g-PAA hydrogels.
  • Synthesis of chitosan-graft-poly(acrylic acid) superabsorbent polymers
  • Analyses of swelling performance using equilibrium swelling and kinetic models
  • Morphological examination using scanning electron microscopy (SEM)
  • Alkali-assisted hydrolysis significantly enhances swelling capacity due to increased ionic carboxylate functionality.
  • Optimal swelling performance is achieved at low crosslinker content.
  • Swelling kinetics align with a pseudo-second-order model, indicating interaction control in water uptake.
  • SEM shows heterogeneous morphologies influenced by processing conditions.

Abstract

ABSTRACT Chitosan‐graft‐poly(acrylic acid) (Cs‐g‐PAA) superabsorbent polymers (SAPs) were synthesized to evaluate the effects of alkali‐assisted hydrolysis and crosslinking density on swelling behavior and structural characteristics. Swelling performance was assessed through equilibrium swelling and kinetic analysis, whereas morphology was examined by scanning electron microscopy (SEM). The results show that alkali‐assisted hydrolysis significantly enhances swelling capacity by increasing ionic carboxylate functionality, with optimal performance at low crosslinker content. Swelling kinetics follow the pseudo‐second‐order model, indicating interaction‐controlled water uptake. SEM observations reveal heterogeneous macroscopic morphologies influenced by processing conditions. Overall, controlled chemical modification is essential for tailoring chitosan‐based SAPs for water‐retention applications.

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Cite This Study

Jayanudin et al. (2026) studied this question.

synapsesocial.com/papers/69af94e870916d39fea4c03chttps://doi.org/10.1002/ceat.70186
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