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March 10, 2026Journal of Applied Polymer Science0 citations

A Novel ZrC – YB 6 ‐Modified PCS Coating Chopped Carbon Fiber/Boron Phenolic Ceramizable Composite Exhibited Outstanding High‐Temperature Resistance

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YXYong XieZWZheng WeiDLDizhi Liu

Key Points

  • The research aims to improve the thermal stability and ablation resistance of carbon fiber/phenolic resin composites.
  • Developed a ceramizable resin-based thermal protection material with PCS coating and ZrC-YB6 modification.
  • Conducted static ablation tests at 1400°C in an oxygen-rich environment.
  • Performed microstructural and phase analysis to assess the ablation mechanism.
  • Achieved a bending strength of 41.82 MPa after static ablation at 1400°C.
  • Reduced linear ablation rate to 0.006 mm/s under a 4.2 MW/m² heat flux.
  • Identified formation of a ceramic-glass-pyrolytic carbon structure that enhances oxidation resistance.

Abstract

ABSTRACT Carbon fiber/phenolic resin composites are commonly employed as ablation heat‐resistant materials in aerospace applications. However, their susceptibility to oxidative degradation and high ablation rates severely limit their development. Therefore, through a synergistic strategy combining fiber coating and matrix modification, a ceramizable resin‐based thermal protection material containing a polycarbosilane (PCS) coating and ZrC–YB 6 was prepared. The research revealed that the ceramizable composite exhibited a bending strength as high as 41.82 MPa after static ablation at 1400°C in an oxygen‐rich environment. Concurrently, after 30 s of ablation under a 4.2 MW/m 2 oxygen‐acetylene heat flux, its linear ablation rate was reduced to 0.006 mm/s, respectively. Through microstructural analysis, phase analysis, and thermodynamic calculations, the ablation mechanism was elucidated. Pyc and ceramic products such as ZrO 2 , ZrB 2 , YSZ, SiC, and SiO 2 form a composite structure of ceramic–glass–pyrolytic carbon on the ablation surface, significantly enhancing the composite's resistance to oxidation corrosion.

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Cite This Study

Xie et al. (2026) studied this question.

synapsesocial.com/papers/69af955970916d39fea4cc4ahttps://doi.org/10.1002/app.70628
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