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March 14, 2026Environmental Progress & Sustainable Energy0 citations

Photocatalytic degradation of 2,4‐ D ichlorophenoxyacetic acid by zero‐valent A g‐modified zinc oxide composite

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FZFabo ZhangYCYu ChenXBXiaoli Bai

Key Points

  • To evaluate the photocatalytic degradation efficiency of 2,4-Dichlorophenoxyacetic acid using modified zinc oxide.
  • Synthesis of zinc oxide supported on Baizilian biochar with simultaneous silver doping.
  • Assessment of photocatalytic activity for 2,4-D degradation using 3% Ag-ZnO/ABC.
  • Measurement of degradation rate and photocatalytic rate constant.
  • Achieved 95.4% degradation of 2,4-D in 50 minutes.
  • Photocatalytic rate constant of 0.06462 min−1, showing significant improvement over pure ZnO.
  • Proposed two plausible degradation pathways based on intermediate identification.

Abstract

Abstract Photocatalytic degradation has emerged as a highly promising and effective approach for the removal of 2,4‐Dichlorophenoxyacetic acid (2,4‐D), a widely used herbicide. In this study, a one‐step calcination method was developed to synthesize zinc oxide (ZnO) supported on Baizilian biochar (ABC) with simultaneous doping of silver (Ag). The ZnO/ABC catalyst incorporating 3% Ag nanoparticles exhibits the highest photocatalytic activity, achieving a 2,4‐D degradation rate of 95.4% within 50 min, exhibiting a photocatalytic rate constant of 0.06462 ± 0.0004 min −1 , which is 3.21 and 1.80 times higher than that of pure ZnO and ZnO/ABC, respectively. Mechanistic investigations revealed that the incorporation of silver nanoparticles reduced the band gap energy of the 3% Ag‐ZnO/ABC system, thereby enhancing the separation efficiency and utilization of photogenerated electrons and holes, leading to increased generation of •O₂ − responsible for organic pollutant degradation. Furthermore, based on the identification of intermediate products, two plausible degradation pathways were proposed.

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Cite This Study

Zhang et al. (2026) studied this question.

synapsesocial.com/papers/69b4b9eb18185d8a39802329https://doi.org/10.1002/ep.70427
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