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March 15, 2026JDS Communications0 citationsOpen Access

UHPLC-HRMS-based screening of purine and pyrimidine metabolites in cow milk collected across four different seasons

MEMichela ErricoGRGabriele RocchettiMLMarco Lapris

Key Points

  • This research aims to evaluate seasonal variations in purine and pyrimidine metabolites in cow milk using untargeted metabolomics.
  • Applied untargeted metabolomics on bulk-tank milk samples from herds in the Po Valley, Italy.
  • Collected samples across four seasons under a standardized feeding regimen.
  • Annotated a total of 82 metabolites related to purine and pyrimidine pathways.
  • Performed multivariate analyses to identify distinct nucleotide profiles by season.
  • Summer and fall showed more distinctive nucleotide profiles compared to spring and winter.
  • Adenosine- and guanosine-related compounds were the main discriminants between seasons.
  • Phosphoribosyl pyrophosphate was identified as a key intermediate in metabolism.
  • Uric acid and allantoin levels remained stable across seasons, while aminoisobutyric acid increased in summer.

Abstract

Milk nucleotides have received little attention compared with other metabolite classes, despite their central role in rumen microbial activity and potential value as markers of nutritional and environmental dynamics.This study applied untargeted metabolomics to screen purine-and pyrimidine-related metabolites in bulk-tank milk collected from dairy herds in the Po Valley (Italy) across 4 seasons under a standardized corn silage-based total mixed ration.A total of 82 metabolites were annotated, with purine and pyrimidine metabolism emerging as central hubs in the milk metabolome and showing connections with amino acid and nitrogen pathways.Multivariate analyses revealed that summer and fall samples had more distinctive nucleotide profiles than spring and winter, with adenosine-and guanosine-related compounds being the main discriminants.Phosphoribosyl pyrophosphate was identified as a key intermediate linking purine and pyrimidine metabolism, while carbamoyl phosphate accumulation in summer highlighted the sensitivity of pyrimidine pathways to environmental stressors.Semiquantitative evaluation of known markers showed stable levels of uric acid and allantoin across seasons, whereas -aminoisobutyric acid, a pyrimidine catabolite, increased in summer.These findings suggest that both pyrimidine and purine metabolism are responsive to seasonal influences under controlled feeding, positioning -aminoisobutyric acid, and potentially carbamoyl phosphate, as candidate tracers of summer-related metabolic adaptations in dairy cows.

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Cite This Study

Errico et al. (2026) studied this question.

synapsesocial.com/papers/69b64c67b42794e3e660dac2https://doi.org/10.3168/jdsc.2025-0924
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