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April 13, 2026Materials Today0 citationsOpen Access

Friction-induced electrochemical activation of platinum group metals via electromechanical coupling

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CLChenxu LiuZZZhaoran ZhuWOWengen Ouyang

Key Points

  • The aim is to explore the effects of friction and electric fields on the reactivity of platinum group metals.
  • Examined PGM reactivity at metal-water interfaces under friction and electric fields.
  • Analyzed the formation of submicron oxide layers on platinum surfaces due to friction.
  • Investigated the role of reduced activation energy in anodic oxidation.
  • Friction coupled with electric fields led to faster formation of oxide layers on platinum.
  • Enhanced anodic oxidation was linked to stress-augmented mechanisms.
  • Nanostructured oxides showed higher electrocatalytic activity than metallic platinum.

Abstract

Platinum group metals (PGMs), long considered chemically inert, exhibit unexpected reactivity at the metal-water interface when subjected to simultaneous friction and electric fields. This tribo-electrochemical coupling unveils a reaction regime fundamentally different from conventional electrochemical or mechanical activation. Here, we demonstrate that friction, coupled with a positive surface potential, drives the rapid formation of submicron oxide layers on platinum surfaces. We propose that friction lowers activation energy barriers and enhances mass transport, thereby accelerating anodic oxidation through a stress-augmented thermally activated mechanism. The resulting nanostructured oxides apparently exhibit higher electrocatalytic activity than that of metallic platinum, offering promising potential for microscale sensors and catalytic microreactors. Notably, this localized oxidation also occurs in other PGMs, indicating a broadly applicable strategy for activating inert metals via electromechanical coupling.

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Cite This Study

Liu et al. (2026) studied this question.

synapsesocial.com/papers/69dc89823afacbeac03eb2b1https://doi.org/10.1016/j.mattod.2026.103323
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