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April 16, 2026European Journal of Organic Chemistry1 citationsOpen Access

1,2,6‐Thiadiazin‐4‐ones: Robust Photocatalysts for the Green Aerobic Oxidation of Sulfides to Sulfoxides

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CKCharikleia I. KaraoustaSSStamatis K. ServiouCSChrysanthi K. Spyropoulou

Key Points

  • To investigate the effectiveness of 1,2,6-thiadiazin-4-ones as photocatalysts for the oxidation of sulfides to sulfoxides.
  • Utilized low catalyst loading (0.01 mol%) for oxidation reactions
  • Employed a 440 nm lamp for photocatalytic irradiation
  • Used molecular oxygen as an oxidant
  • Tested a variety of sulfides including alkyl-aryl, dialkyl, and diaryl types
  • Successfully oxidized sulfides to sulfoxides with high chemoselectivity
  • Achieved rapid reaction times under mild conditions
  • Indicated practical relevance for pharmaceutical synthesis, particularly for compounds like modafinil and sulforaphane

Abstract

The chemoselective oxidation of sulfides to sulfoxides is accomplished using a new family of photocatalysts, namely 1,2,6‐thiadiazin‐4‐ones. Utilizing a low catalyst loading (0.01 mol%), a 440 nm lamp as the irradiation source, and molecular oxygen as the oxidant, this rapid method is applicable to a broad range of alkyl‐aryl, dialkyl, and diaryl sulfides. Additionally, the method demonstrates practical relevance for the industrially significant synthesis of pharmaceutical compounds, including modafinil and sulforaphane.

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Cite This Study

Karaousta et al. (2026) studied this question.

synapsesocial.com/papers/69e07c972f7e8953b7cbdd24https://doi.org/10.1002/ejoc.70448
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