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April 16, 2026International Journal of Chemical Kinetics0 citations

Activity Based Model Development for Esterification Reaction of‐Propionic Acid and n‐Propyl Alcohol With Solid Acidic Catalyst

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TVTirumalaiah VelivalaRRRukmini RayannagariMMMallaiah Mekala

Key Points

  • To develop a kinetic model for the esterification reaction of n-propionic acid and n-propyl alcohol using Indion 140 catalyst.
  • Conducted esterification in an isothermal batch reactor
  • Varying temperature from 333 to 353 K
  • Catalyst loading ranged from 0.01 to 0.03 g/cc
  • Mole ratio of reactants varied from 1:1 to 1:6
  • Determined kinetic parameters from experimental data using a second-order pseudo-homogeneous model.
  • The reaction was found to be kinetic controlled, not mass transfer controlled.
  • A second-order pseudo-homogeneous kinetic rate equation effectively described the reaction.
  • Activation energies and rate constants were determined using Arrhenius plots.
  • Simulation results aligned closely with experimental data, supporting the new model.

Abstract

ABSTRACT The esterification reaction of n‐propyl alcohol with n‐propionic acid using Indion 140 solid catalyst is carried out in an isothermal batch reactor to produce n‐propyl propionate and water. The reaction temperature is maintained in the range of 333–353 K and the catalyst loading varies from 0.01 to 0.03 g/cc. The mole ratio of n‐propionic acid and n‐propyl alcohol varies from 1:1 to 1:6. The influence of various parameters such as temperature, catalyst loading, initial reactant molar ratio, catalyst size, and agitation speed on the reaction rate are investigated. From the experimental results, it is observed that the reaction is kinetic controlled rather than mass transfer controlled. A second‐order pseudo‐homogeneous kinetic rate equation is used to fit the experimental data. The activation energies and forward reaction rate constants are obtained from the Arrhenius plot. The comparison of the simulation results with the experimental data indicates the second‐order pseudo‐homogeneous non‐ideal kinetic model better describes the behavior of the esterification reaction. The rate equation thus developed in this work can be used in modeling and design of catalytic distillation involving esterification of propionic acid with propanol.

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Cite This Study

Velivala et al. (2026) studied this question.

synapsesocial.com/papers/69e07e242f7e8953b7cbf105https://doi.org/10.1002/kin.70065
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