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April 23, 2026Polymers0 citationsOpen Access

The Influence of the Flow Direction of KOH Solutions on the Measurement of Dissolved Hydrogen Permeability Through Alkaline Water Electrolysis Membranes

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JLJun Hyun LimJHJin Pyo HwangEOEuntaek Oh

Key Points

  • The research aims to improve measurement techniques for hydrogen permeability through AWE membranes.
  • Proposes a cross-flow measurement methodology for AWE membranes.
  • Compares the cross-flow approach to traditional dead-end configurations.
  • Examines the impact on impurity accumulation and measurement reliability.
  • The cross-flow methodology reduces impurity accumulation, enhancing measurement accuracy.
  • Improved performance is observed for dense anion exchange membranes with low permeability.
  • Findings suggest significant advantages in measurement reliability and reproducibility.

Abstract

Alkaline water electrolysis (AWE) is a pivotal technology for sustainable hydrogen production. However, hydrogen permeation through its membranes remains a critical concern, as excessive gas crossover can lead to the formation of explosive mixtures and pose severe safety hazards. While conventional measurement techniques, such as pressure drop and electrochemical methods, are suitable for porous membranes, they exhibit inherent limitations when applied to dense membranes such as anion exchange membranes. This study proposes a cross-flow measurement methodology applicable to all types of AWE membranes. Unlike traditional dead-end configurations, the cross-flow approach effectively mitigates impurity accumulation and maintains a continuous electrolyte flow parallel to the membrane surface. This configuration ensures uniform electrolyte distribution, minimizes local concentration and pressure fluctuations, and enhances measurement reliability and reproducibility relative to the conventional dead-end flow. Furthermore, the methodology ensures accurate and reproducible measurements, demonstrating enhanced detection capability for dense membranes with intrinsically low permeability by mitigating fouling and concentration polarization effects. These findings provide a robust framework for the development of high-performance membranes designed to suppress dissolved hydrogen permeability.

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Cite This Study

Lim et al. (2026) studied this question.

synapsesocial.com/papers/69e9bb6285696592c86ed0c7https://doi.org/10.3390/polym18081006
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