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April 29, 2026Small0 citations

In Situ Surface Reconstruction and Carbon Encapsulation for High‐Performance Pt‐Lean Catalysts beyond Conventional Core–Shell Designs (Small 24/2026)

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JMJiho MinJLJeong Hee LeeKKKeonwoo Ko

Key Points

  • To investigate a new strategy for developing high-performance catalytic structures with reduced platinum usage.
  • In-situ one-step synthesis of Pt–3d alloy nanoparticles
  • Formation of porous carbon shell surrounding the catalysts
  • Assessment of catalyst durability and activity during the oxygen reduction reaction
  • The synthesized catalysts showed enhanced oxygen reduction activity compared to conventional designs.
  • Catalysts maintained long-term durability with reduced platinum usage.
  • This method offers a practical pathway for developing low-cost, high-performance catalysts.

Abstract

Oxygen Reduction Reaction An in-situ one-step synthesis simultaneously induces Pt surface segregation and forms a porous carbon shell on Pt–3d alloy nanoparticles. The resulting structure stabilizes the catalyst while maintaining high oxygen reduction reaction activity and long-term durability, enabling reduced Pt usage without sacrificing fuel-cell activity. This promising strategy offers a practical pathway toward low-cost, high-performance catalysts beyond conventional core–shell structures. More in the Research Article (e11516), Yun Sik Kang, Joseph T. Hupp, Sung Jong Yoo, Namgee Jung, and co-workers.

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Cite This Study

Min et al. (2026) studied this question.

synapsesocial.com/papers/69f19ff5edf4b46824806a3dhttps://doi.org/10.1002/smll.73116
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