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May 1, 2026Journal of the American Chemical Society1 citations

Interlayer Electronic Coupling Breaks the *OH Desorption Limitation in Single-Atom Oxygen Reduction Catalysts

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ZLZengyuan LiWMWenhao MiaoQHQi Huang

Key Points

  • The aim is to investigate how interlayer electronic coupling affects the performance of single-atom oxygen reduction catalysts.
  • Identification of interlayer electronic coupling as a design parameter for catalysts
  • Comparison with commercial platinum-based catalysts for performance assessment
  • Examination of long-term cycling stability
  • Interlayer electronic coupling allows access to previously inaccessible reaction energetics.
  • Catalysts exhibit enhanced stability and performance compared to traditional platinum-based alternatives.

Abstract

Zn, and long-term cycling stability, surpassing commercial 20 wt % Pt/C. This work identifies interlayer electronic coupling as an orthogonal design dimension to conventional coordination engineering, enabling access to reaction energetics that are intrinsically inaccessible in planar single-atom catalysts.

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Cite This Study

Li et al. (2026) studied this question.

synapsesocial.com/papers/69f44464967e944ac55675cdhttps://doi.org/10.1021/jacs.6c02011
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