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May 7, 2026Industrial & Engineering Chemistry Research0 citations

Interfacial Tension Response of Crude Oil–Brine Systems to Low-Voltage Direct and Pulsed Electric Fields

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NHNegin Ghaderi HayatiJSJavad SaienFJFarnaz Jafari

Key Points

  • The study aims to analyze how low-voltage electric fields affect the interfacial tension in crude oil-brine systems with different salt concentrations.
  • IFT was measured using a pendant drop device with parallel electrodes at 1–3 V/cm and 100–1000 Hz frequencies.
  • Effects of square-wave pulsed electric fields were assessed with brine concentrations of 0.001–0.005 mol/dm3.
  • Asphaltenes were characterized to study the role of indigenous surfactants.
  • Square-wave pulsed electric field (3 V/cm, 600 Hz) reduced IFT by 82.5% (from 27.5 to 4.8 mN/m) for NaCl (0.005 mol/dm3).
  • Divalent salts (MgCl2 and Na2SO4) showed similar reductions of 82.7% and 84.7%, respectively.
  • Direct and sinusoidal waves were effective, but with less impact than the square wave.

Abstract

Electro-assisted enhanced oil recovery (EEOR) is an emerging technology that could significantly improve sweep efficiency. The aim of the present study was to scrutinize the simultaneous use of monovalent and divalent salts under low-voltage electric fields of direct and pulsed (sinusoidal and square waves) as a novel approach for reducing the IFT of crude oil–brine systems. IFTs were measured using a pendant drop device featuring parallel electrodes for electric field application at strengths of 1–3 V/cm and frequencies of 100–1000 Hz, with brine concentrations of 0.001–0.005 mol/dm3. Applying a square-wave pulsed electric field (3 V/cm, 600 Hz) brought about IFT changes from 27.5, 27.1, and 26.1 mN/m to 4.8, 4.7, and 4.0 mN/m at 0.005 mol/dm3 of NaCl, MgCl2, and Na2SO4, i.e., 82.5, 82.7, and 84.7% reductions, respectively. The IFT reduction corresponded to the boosted ion–dipole interactions under electro-hydrodynamic (EHD) effects, promoting adsorption of indigenous natural surfactants and interfacial instabilities induced by switching poles. Direct and sinusoidal waves were also effective but inferior to the square wave. Asphaltenes were precipitated and characterized to assess the role of present indigenous surfactants. Further, the IFT data were precisely adapted with the Young–Laplace equation combined with a developed correction factor as a function of involved parameters.

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Cite This Study

Hayati et al. (2026) studied this question.

synapsesocial.com/papers/69fc2b608b49bacb8b347898https://doi.org/10.1021/acs.iecr.6c00095
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