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May 14, 2026Advanced Functional Materials0 citations

Optimizing Interfaces Between Mixed‐Halide Perovskite Nanocrystals and Encapsulants Through Ligand Engineering for Stable White Light‐Emitting Diode Applications

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YJYongqiang JiZCZhiqiang ChenYWYuquan Wang

Key Points

  • This research aims to enhance the stability and luminescence of mixed-halide perovskite nanocrystals for white light-emitting diodes (WLEDs).
  • Employed multifunctional ligand 8-amino-1-naphthalenesulfonic acid (ANA) with SBA-15 as encapsulant.
  • Reduced defect density and recombination loss through optimized interface interactions.
  • Analyzed luminescence properties and device lifetime of WLEDs using these modified PeNCs.
  • Photoluminescence quantum yield (PLQY) exceeded 90%.
  • WLED devices demonstrated a T50 (device half-life) of 320 hours.
  • Improved stability under water, heat, and ultraviolet light conditions compared to control samples.

Abstract

ABSTRACT All inorganic mixed‐halide perovskite nanocrystals (PeNCs) have demonstrated great potential in display applications. However, poor stabilities of PeNCs under water, heat, and light strictly hinder their commercialization. Herein, by simultaneously employing a multifunctional ligand molecule, 8‐amino‐1‐naphthalenesulfonic acid (ANA), as well as SBA‐15 as the encapsulant, interactions at the interface of PeNCs/SBA‐15 were enhanced, which contributes to reduced defect density, suppressed recombination loss, and enhanced luminescence properties with a high photoluminescence quantum yield (PLQY) of over 90%. Moreover, target PeNCs exhibited much enhanced water, heat, and ultraviolet light stabilities compared to control samples. More importantly, white light‐emitting diode (WLED) devices based on these optimized PeNCs were fabricated, which demonstrated high color purity and a decent device half lifetime (T 50 ) of 320 h. This work highlights the significance of optimizing interfaces at PeNCs/encapsulant and is expected to promote future developments of stable PeNCs and LED devices.

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Cite This Study

Ji et al. (2026) studied this question.

synapsesocial.com/papers/6a05680ea550a87e60a205c1https://doi.org/10.1002/adfm.202528164
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