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May 17, 2026Drug Delivery Letters0 citations

Innovations and Bottlenecks in Thermosensitive Polymer Hydrogels for Nose-to-Brain Delivery: A Comprehensive Review

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AKAkshay KumarSVSushma VermaAMAbhilasha Mishra

Key Points

  • This review aims to discuss the advancements and challenges in thermosensitive hydrogels for nose-to-brain delivery of drugs targeting the central nervous system.
  • Comprehensive analysis of literature on thermosensitive hydrogels and their components for drug delivery to the brain.
  • Evaluation of innovations like chitosan-poloxamer blends and PNIPAM-PEG copolymers in enhancing drug delivery.
  • Discussion of challenges, including batch variability and regulatory hurdles affecting clinical translation.
  • Innovative formulations showed improved brain exposure and targeting efficiency in preclinical studies.
  • Integration of nanotechnology enhanced targeting specificity and enabled on-demand drug release.
  • Identified bottlenecks include variability in gelation kinetics and the need for standardized regulatory pathways.

Abstract

Abstract: Thermosensitive hydrogels have emerged as a transformative platform for nose-to-brain drug delivery, allowing a non-invasive approach to bypass the blood-brain barrier and ad-dress the growing worldwide burden of neurological diseases. This article discusses innovations and bottlenecks in thermosensitive polymer hydrogel systems for intranasal central nervous sys-tem (CNS) targeting. Recent breakthroughs include composite polymer systems such as chitosan-poloxamer blends and PNIPAM-PEG copolymers that provide accurate lower critical solution temperature control (32-34°C), increased mucoadhesion, and sustained release. Optimized formu-lations have demonstrated improved drug loading, prolonged nasal residence, and substantial en-hancement of brain exposure and targeting efficiency in preclinical studies. Nanotechnology inte-gration-which includes lipid nanocapsules, polymeric micelles, and ligand-functionalized carri-ers-further improves targeting specificity, while multi-responsive structures (pH, enzyme, and re-dox-sensitive) enable on-demand release. Despite these gains, translation is hindered by batch variability, temperature-dependent stability, limited hydrophilic drug loading, variable gelation kinetics, and a lack of validated human-relevant preclinical models. Regulatory pathways also lack uniform evaluation standards, impeding scale-up and GMP standardization. Future progress will depend on integrating predictive human organoid and physiologically based pharmacokinetic platforms, rigorous long-term safety frameworks, and strategic intellectual property management to convert laboratory discoveries into clinically feasible therapies for Alzheimer’s, Parkinson’s, epilepsy, and related CNS disorders.

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Kumar et al. (2026) studied this question.

synapsesocial.com/papers/6a095c5d7880e6d24efe26d5https://doi.org/10.2174/0122103031469252260423141956
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