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May 27, 2026ACS Applied Materials & Interfaces0 citations

Low-Transmission-Loss Optical Waveguide Devices of Polyimides with Trifluoromethoxy-Enhanced Ultrahigh Refractive Index for Short-Distance Optical Communication

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XYXiaoliang YuYZYuxiao ZhaoLTLuyao Tian

Key Points

  • The aim is to develop high-performance optical transmission media using polyimides with enhanced refractive properties.
  • Developed ternary copolymerized polyimides via two-step thermal imidization.
  • Introduced trifluoromethoxy groups to improve optical properties.
  • Evaluated performance under standard optical communication wavelengths (1310 and 1550 nm).
  • Polymers achieved an ultrahigh refractive index above 1.8.
  • Demonstrated an ultralow birefringence of 0.003.
  • Showed very weak signal attenuation and absorption behaviors, indicating strong potential for optical communication.

Abstract

Short-distance optical communication technology has been promoted to a crucial position with the rapid development of network systems centered around data, which inevitably leads to the urgency of developing a high-performance optical transmission medium. To address these requirements, several ternary copolymerized polyimides, known as high-performance engineering plastics, are developed through the most common two-step thermal imidization strategy. The introduction of trifluoromethoxy (−OCF3) groups provides polymers with an ultrahigh refractive index above 1.8 under the common observation conditions of communication wavelengths, as well as an ultralow birefringence of 0.003. More importantly, under the chief band of optical fiber communication at 1310 and 1550 nm, generated by modulated lasers, these polymers show very weak light absorption and signal attenuation behaviors, thereby demonstrating huge potential in the field of optical waveguide device development. Additionally, considering the extremely low moisture absorption of the polymers, these transparent polyimides with high refractive index are expected to be fundamental material candidates in many fields, such as optical communication, the Internet of Things, 5G transmission, and other advanced technologies in extreme environments.

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Cite This Study

Yu et al. (2026) studied this question.

synapsesocial.com/papers/6a168b160c924ddd1bd59f76https://doi.org/10.1021/acsami.6c07517
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