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May 31, 2026ChemPhysChem0 citationsOpen Access

Heterogeneous Fenton Degradation of Nalidixic Acid on Fe(II)‐Sorbed Maghemite, as Probed by In Situ Attenuated Total Reflectance‐Fourier Transform Infrared Spectroscopy

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AFAna Carolina Schuh FrantzMRMbolantenaina Rakotomalala RobinsonAMAlberto Mezzetti

Key Points

  • This research aims to explore the degradation mechanisms of nalidixic acid using heterogeneous Fenton reactions with Fe(II)-sorbed maghemite.
  • Utilized heterogeneous Fenton reactions with Fe(II)-sorbed maghemite as a catalyst.
  • Applied in situ attenuated total reflectance-Fourier transform infrared spectroscopy to monitor degradation.
  • Investigated the influence of surface loading of nalidixic acid and Fe(II) on reaction efficiency.
  • Key spectral changes observed indicate the formation of degradation products and a ring-opening in initial degradation steps.
  • The efficiency of reactions varies with the surface loading of nalidixic acid and Fe(II).
  • Findings contribute to understanding advanced oxidation processes for antibiotic degradation.

Abstract

The degradation of nalidixic acid (NAL) via heterogeneous Fenton reactions is investigated using Fe(II)‐sorbed maghemite (Mh) as catalyst. The Fenton reaction is triggered by hydrogen peroxide (H 2 O 2 ) and in situ attenuated total reflectance‐Fourier transform infrared spectroscopy is employed to monitor the evolution of the NAL spectrum, providing insights into the degradation mechanisms at the molecular level. Key spectral changes are observed, indicating the formation of degradation products and suggesting a ring‐opening in the first degradation steps. The efficiency of the reactions is influenced by the surface loading of NAL and Fe(II) on the substrates. This work contributes to the understanding of advanced oxidation processes for antibiotic degradation relying on cost‐effective remediation techniques.

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Cite This Study

Frantz et al. (2026) studied this question.

synapsesocial.com/papers/6a1bd2375783ba022b6fda7fhttps://doi.org/10.1002/cphc.202500857
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