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June 4, 2026ChemistryEurope0 citationsOpen Access

Hydrogenative Conversion of C5 Biomass Feedstock Furoic Acid to δ‐Valerolactone on Pt‐Loaded Silicoaluminophosphate

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HIHaruro IshitaniTUTakashi UemuraTKTomoya Kawase

Key Points

  • This research aims to assess the effectiveness of Pt catalysts for converting furoic acid to δ-valerolactone.
  • Developed Pt catalysts supported on silicoaluminophosphate.
  • Evaluated catalyst performance under mild reaction conditions for furoic acid conversion.
  • Conducted continuous flow reactions to test productivity and selectivity.
  • Catalysts showed high activity and selectivity for δ-valerolactone production.
  • High dispersion of Pt nanoparticles attributed to the support's porous structure enhanced reaction performance.
  • Catalysts demonstrated efficient site-selective partial hydrogenation and selective Csp2–O bond cleavage.

Abstract

Novel Pt catalysts supported on zeolitic silicoaluminophosphate were developed, and their performance was evaluated for the hydrogenative conversion of furoic acid under mild reaction conditions. The catalysts exhibited high activity and selectivity for the conversion to δ ‐valerolactone, a versatile intermediate for the production of polyesters from woody biomass. Catalyst characterization revealed that the high activity is attributed to the high dispersion of Pt nanoparticles, which is facilitated by the porous structure of the support. Further investigation using analogs and intermediates provided insights into the reaction mechanism, suggesting site‐selective partial hydrogenation followed by selective Csp 2 –O bond cleavage. The developed catalyst was successfully applied in a continuous flow reaction, demonstrating high productivity and selective conversion.

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Cite This Study

Ishitani et al. (2026) studied this question.

synapsesocial.com/papers/6a2116fad499ed480b16fe19https://doi.org/10.1002/ceur.202600003
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